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Weekly composite, bulk air was sampled with respect to wind speed and direction from January 1996 through December 1997 in one urban and two agricultural locations in Sacramento County, California. The sampling sites were located along a north-south transect, the dominant directions of the prevailing winds. The samples were analyzed for a variety of current-use pesticides, including dormant orchard spray insecticides and rice herbicides. A variety of pesticides were detected throughout the year, predominantly chlorpyrifos, diazinon, and trifluralin. The data obtained during the winter and spring suggest that some pesticides used in agricultural areas become airborne and may be transported into the urban area. Confirmation of this drift is difficult, however, because these three predominant pesticides, as well as other detected pesticides, also are heavily used in the urban environment. The spring data clearly show that molinate and thiobencarb, two herbicides used only in rice production, do drift into the urban environment.
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Water quality data collected at 17 sites in urbanized and rural parts of the 438 sq km Irondequoit Creek basin from July 1980 through August 1981 were used to compute annual loads of eight selected constituents. Of the total annual loads of these constituents, 50 to 70% was transported to Irondequoit Bay during a 3.5-month period from late January to early May. Of six mixed-land-use subbasins, the two most highly urbanized had the highest loads of all constituents. Of the four sites representing single land uses, the high density residential site and the housing construction site had the highest loads of all constituents except cadmium. A rainfall-runoff model was used to predict quantity and quality of storm runoff leaving one commercial site, two residential sites, and a large mixed-land-use subbasin. Predicted volume and peak discharges were within 10 to 30% of the measured values; predicted runoff loads of most constituents were within 40 to 60% of measured values. Stormflow modification in the Irondequoit Creek wetlands by two hypothetical control structures was simulated. Results indicate that outflow from the upper wetland could be decreased and stormflows dispersed to a greater part of the upper wetland to increase retention of suspended solids and associated chemical constituents.
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All of the rain samples during the growing season had detectable quantities of at least one pesticide, but most of the pesticides were only infrequently observed. The most frequently detected compounds were the herbicides alachlor, atrazine, cyanazine, and metolachlor, and in 1994, its first year of registration, acetochlor. Peak concentrations of most herbicides in rainfall occurred shortly after their application periods in the spring. Peak concentrations of most of the insecticides occurred later in the summer. The majority of the wet depositional flux of pesticides occurred between early May and October. The annual wet depositional flux of pesticides is 5 orders of magnitude less than is the "annual flux" normally applied on an agricultural field, although some of the pesticides in rain are deposited in areas far removed from agricultural fields. The annual variability in pesticide deposition can be explained by year-to-year differences in climate and pesticide use patterns. The one sampling site (Lamberton) that was in an area dominated by row crop agriculture showed a significantly greater annual flux than the other four sampling sites that were in areas of either urbanization or less intensive agricultural. Regional deposition, away from a local source, can be inferred from these four sites because they have annual pesticide fluxes that are very similar for any given year. The observation of agricultural pesticides (not registered for home and garden use) in rain and storm runoff in the urban area indicates their transport from areas of agricultural use. Urban areas may be the best locations for assessing changes in regional use and deposition of agricultural pesticides. The pesticide fluxes in the streams out of the small three watersheds was compared to the pesticide flux into the watersheds in rain. The data indicate that flux into the watersheds from the rain is generally much greater than the flux from the watersheds in the streams. Therefore, a large fraction of the pesticides deposited in rain is retained within the watersheds. For the urban area, this is on the order of 98 percent for the four most commonly observed herbicides in rain and runoff.
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This white paper demonstrates five points: (1) The lack of robust measurements of the vertical gradients of natural boundary layers and transport fluxes on other planetary bodies precludes adequate estimation of aeolian and other meteorological processes throughout our Solar System (§1). (2) Thus, there exist critical knowledge gaps within high-priority planetary science questions that motivate the need for in situ aeolian and other meteorological measurements on an extraterrestrial surface (§2). (3) Such measurements would be timely, because they will greatly enhance the utility of existing climate data/models, while also contributing to improved design, safety, and effectiveness of near-future missions (§3). (4) Acquisition of these next-generation measurements from Mars is technologically feasible within the coming decade (including via small spacecraft) (§4, 6) and (5) such measurements would also significantly contribute towards addressing key Mars science questions (§5). Our implicit recommendation is that this type of in situ science be considered in definition of high-priority planetary science questions and prioritization of mission concepts.
Twenty-seven years of data from midcontinent wetlands indicate that the response of these wetlands to extremes in precipitation-drought and deluge-persists beyond the extreme events. Chemical changes transcend such simple relations as increased salinity during dry periods because drought provides mechanisms for removal of salt by deflation and seepage to groundwater. Inundation of vegetation zones including rooted or floating mats of cattail (Typha glauca) can stimulate sulfate reduction and shift the anion balance from sulfate to bicarbonate dominance. Disruptions in the circulation of moisture-laden air masses over the midcontinent, as in the drought of 1988 and the deluge of 1993, have a major effect on these wetlands, which are representatives of the primary waterfowl breeding habitat of the continent.
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