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USGS2006

Organic geochemistry - A retrospective of its first 70 years

Organic geochemistry had its origin in the early part of the 20th century when organic chemists and geologists realized that detailed information on the organic materials in sediments and rocks was scientifically interesting and of practical importance. The generally acknowledged "father" of organic geochemistry is Alfred E. Treibs (1899-1983), who discovered and described, in 1936, porphyrin pigments in shale, coal, and crude oil, and traced the source of these molecules to their biological precursors. Thus, the year 1936 marks the beginning of organic geochemistry. However, formal organization of organic geochemistry dates from 1959 when the Organic Geochemistry Division (OGD) of The Geochemical Society was founded in the United States, followed 22 years later (1981) by the establishment of the European Association of Organic Geochemists (EAOG). Organic geochemistry (1) has its own journal, Organic Geochemistry (beginning in 1979) which, since 1988, is the official journal of the EAOG, (2) convenes two major conferences [International Meeting on Organic Geochemistry (IMOG), since 1962, and Gordon Research Conferences on Organic Geochemistry (GRC), since 1968] in alternate years, and (3) is the subject matter of several textbooks. Organic geochemistry is now a widely recognized geoscience in which organic chemistry has contributed significantly not only to geology (i.e., petroleum geochemistry, molecular stratigraphy) and biology (i.e., biogeochemistry), but also to other disciplines, such as chemical oceanography, environmental science, hydrology, biochemical ecology, archaeology, and cosmochemistry.

Conference Paper↗
USGS2006

Storm-induced redistribution of deepwater sediments in Lake Ontario

High-resolution seismic reflection profiles, side-scan sonar profiles, and surface sediment analyses for grain size (% sand, silt & clay), total organic carbon content, and carbonate content along shore-perpendicular transects offshore of Olcott and Rochester in Lake Ontario were utilized to investigate cm-thick sands or absence of deep-water postglacial sediments in water depths of 130 to 165 m. These deepwater sands were observed as each transect approached and occupied the "sills," identified by earlier researchers, between the three deepest basins of the lake. The results reveal thin (0 to 5-cm) postglacial sediments, lake floor lineations, and sand-rich, organic, and carbonate poor sediments at the deepwater sites (> 130 m) along both transects at depths significantly below wave base, epilimnetic currents, and internal wave activity. These sediments are anomalous compared to shallower sediments observed in this study and deeper sediments reported by earlier research, and are interpreted to indicate winnowing and resuspension of the postglacial muds. We hypothesize that the mid-lake confluence of the two-gyre surface current system set up by strong storm events extends down to the lake floor when the lake is isothermal, and resuspends and winnows lake floor sediment at these locations. Furthermore, we believe that sedimentation is more likely to be influenced by bottom currents at these at these sites than in the deeper basins because these sites are located on bathymetric highs between deeper depositional basins of the lake, and the bathymetric constriction may intensify any bottom current activity at these sites.

Journal of Great Lakes Research↗
USGS2016

Internal loading of phosphorus in western Lake Erie

This study applied eight techniques to obtain estimates of the diffusive flux of phosphorus (P) from bottom sediments throughout the western basin of Lake Erie. The flux was quantified from both aerobic and anaerobic incubations of whole cores; by monitoring the water encapsulated in bottom chambers; from pore water concentration profiles measured with a phosphate microelectrode, a diffusive equilibrium in thin films (DET) hydrogel, and expressed pore waters; and from mass balance and biogeochemical diagenetic models. Fluxes under aerobic conditions at summertime temperatures averaged 1.35 mg P/m 2 /day and displayed spatial variability on scales as small as a centimeter. Using two different temperature correction factors, the flux was adjusted to mean annual temperature yielding average annual fluxes of 0.43–0.91 mg P/m 2 /day and a western basin-wide total of 378–808 Mg P/year as the diffusive flux from sediments. This is 3–7% of the 11,000 Mg P/year International Joint Commission (IJC) target load for phosphorus delivery to Lake Erie from external sources. Using these average aerobic fluxes, the sediment contributes 3.0–6.3 μg P/L as a background internal contribution that represents 20–42% of the IJC Target Concentration of 15 μg P/L for the western basin. The implication is that this internal diffusive recycling of P is unlikely to trigger cyanobacterial blooms by itself but is sufficiently large to cause blooms when combined with external loads. This background flux may be also responsible for delayed response of the lake to any decrease in the external loading.

Lake Erie↗
USGS2013

Emerging methods for the study of coastal ecosystem landscape structure and change

Coastal landscapes are heterogeneous, dynamic, and evolve over a range of time scales due to intertwined climatic, geologic, hydrologic, biologic, and meteorological processes, and are also heavily impacted by human development, commercial activities, and resource extraction. A diversity of complex coastal systems around the globe, spanning glaciated shorelines to tropical atolls, wetlands, and barrier islands are responding to multiple human and natural drivers. Interdisciplinary research based on remote-sensing observations linked to process studies and models is required to understand coastal ecosystem landscape structure and change. Moreover, new techniques for coastal mapping and monitoring are increasingly serving the needs of policy-makers and resource managers across local, regional, and national scales. Emerging remote-sensing methods associated with a diversity of instruments and platforms are a key enabling element of integrated coastal ecosystem studies. These investigations require both targeted and synoptic mapping, and involve the monitoring of formative processes such as hydrodynamics, sediment transport, erosion, accretion, flooding, habitat modification, land-cover change, and biogeochemical fluxes.

International Journal of Remote Sensing↗
USGS1995

Mudflow generated by retrogressive slope failure, Santa Barbara Basin, California continental borderland

The morphology and internal geometry of a mudflow deposit on the mainland slope of the Santa Barbara Basin are defined using high-resolution seismic-reflection data in combination with core samples. Sediment failure occurred on a 4 degrees slope in the uppermost part of late Quaternary well-bedded slope deposits. The failure zone extends from water depths of 374-510 m near the base of slope, occupies an area of 4 km 2 , and involved the translation of 0.01-0.02 km 3 of sediment. Major geomorphic features of the mudflow deposit include a headscarp 6-8 m high, a scar 50-700 m wide, and a main body 1 km long and 12 m thick. The hummocky surface of the mudflow deposits, their chaotic internal structure, and the bulbous toe tapering upslope to a thin tail are consistent with mass flow involving extensive internal deformation. Sediment failed in stages, ending with upslope retrogressive retreat of the headwall along the east side of the failure zone. Known sedimentation rates of 0.8-1.4 m/k.y., as well as the presence of a thin (0.15-0.5 m thick) sediment cap resting atop the scar surface, indicate that the failure probably occurred within the past few centuries. A geotechnical analysis incorporating the results of both static and dynamic triaxial strength tests shows that the failure was probably caused by a strong (M nearly equal 7.5) nearby earthquake. The weakened sediment that remained after earthquake shaking continued to flow down the gentle basin slope under the stresses generated by gravity alone. The analysis also shows that much of the slope sediment is marginally stable and that additional mudflows will probably occur during future strong seismic shaking.

California↗
USGS2006

Metallogeny of the Great Basin: Crustal evolution, fluid flow, and ore deposits

The Great Basin physiographic province in the Western United States contains a diverse assortment of world-class ore deposits. It currently (2006) is the world’s second leading producer of gold, contains large silver and base metal (Cu, Zn, Pb, Mo, W) deposits, a variety of other important metallic (Fe, Ni, Be, REE’s, Hg, PGE) and industrial mineral (diatomite, barite, perlite, kaolinite, gallium) resources, as well as petroleum and geothermal energy resources. Ore deposits are most numerous and largest in size in linear mineral belts with complex geology. U.S. Geological Survey (USGS) scientists are in the final year of a research project initiated in the fall of 2001 to increase understanding of relations between crustal evolution, fluid flow, and ore deposits in the Great Basin. Because of its substantial past and current mineral production, this region has been the focus of numerous investigations over the past century and is the site of ongoing research by industry, academia, and state agencies. A variety of geoinformatic tools was used to organize, reinterpret, and display, in space and time, the large amounts of geologic, geophysical, geochemical, and hydrologic information deemed pertinent to this problem. This information, in combination with concentrated research on (1) critical aspects of the geologic history, (2) an area in northern Nevada that encompasses the major mineral belts, and (3) important mining districts and deposits, is producing new insights about the interplay between key tectonic events, hydrothermal fluid flow, and ore genesis in mineral belts. The results suggest that the Archean to Holocene history of the Great Basin was punctuated by several tectonic events that caused fluids of different origins (sea water, basinal brine, meteoric water, metamorphic water, magmatic water) to move through the crust. Basement faults reactivated during these events localized deformation, sedimentation, magmatism, and hydrothermal fluid flow in overlying rocks to form mineral belts that contain ore deposits of different types and ages that are locally superimposed (demonstrating inheritance). Fluid flow in these systems also was influenced by the distribution of permeable lithologies and paleotopographic highs and lows. Hydrothermal fluids evolved from their initial chemistries towards compositions that reflect the ƒ O 2 and ƒ S 2 buffering capacity of, and the ligands and metals present in, the rocks (±older mineralization) through which they moved. In northern Nevada, where gold deposits are relatively common, carbonaceous, pyritic strata buffered fluids of diverse origins to H 2 S-rich compositions so they could transport gold repeatedly over Paleozoic-Cenozoic time (convergent evolution). Ore formed where metal-laden fluids encountered effective physicochemical traps. Maps of Neogene basin fill and erosion surfaces identify areas where preexisting ore deposits have been progressively exposed or concealed. Comparisons with analogous terrains and deposit types in other parts of the world provide global context. The initial findings and some of the databases, geologic maps, sections, reconstructions, hydrogeologic models, topical syntheses, regional overviews, short courses, field guides, and deposit comparisons produced by project staff and associated managers, contractors, and collaborators have been presented in numerous abstracts, symposia, USGS publications, and professional journals over the last 5 years (see the extensive bibliography). Notable among these was the 2005 Geological Society of Nevada symposium in Reno, Nevada, and the 2005 Geological Society of America annual meeting in Salt Lake City, Utah, where project results were presented to audiences from around the nation and world. The final results of the project will be submitted for publication in 2007 to appropriate USGS and professional journals. A special issue of GEOSPHERE, scheduled for publication in 2007, will be devoted to the results of this project and related work. This special issue will reach an international audience and be available worldwide on the internet. Much of the research for this project has concentrated on areas that will receive the focused attention of the mining industry in the future. As such, the data and interpretations generated by this project have direct use for land-use managers in Federal, State, and local agencies. Improved hydrogeologic models developed by this project will considerably enhance ongoing and future water resource investigations in the region. The increased understanding of when, where, and how hydrothermal systems produce significant economic deposits has direct uses for mineral exploration and for future USGS mineral resource assessments in the Great Basin and other parts of the world.

Great Basin↗
USGS2008

The A and m coefficients in the Bruun/Dean equilibrium profile equation seen from the Arctic

The Bruun/Dean relation between water depth and distance from the shore with a constant profile shape factor is widely used to describe shoreface profiles in temperate environments. However, it has been shown that the sediment scale parameter (A) and the profile shape factor (m) are interrelated variables. An analysis of 63 Arctic erosional shoreface profiles shows that both coefficients are highly variable. Relative frequency of the average m value is only 16% by the class width 0.1. No other m value frequency exceeds 21%. Therefore, there is insufficient reason to use average m to characterize Arctic shoreface profile shape. The shape of each profile has a definite combination of A and m values. Coefficients A and m show a distinct inverse relationship, as in temperate climate. A dependence of m values on coastal sediment grain size is seen, and m decreases with increasing grain size. With constant m = 0.67, parameter A obtains a dimension unit m1/3. But A equals the water depth in meters 1 m from the water edge. This fact and the variability of parameter m testify that the Bruun/Dean equation is essentially an empirical formula. There is no need to give any measurement unit to parameter A. But the International System of Units (SI) has to be used in applying the Bruun/Dean equation for shoreface profiles. A comparison of the shape of Arctic shoreface profiles with those of temperate environments shows surprising similarity. Therefore, the conclusions reached in this Arctic paper seem to apply also to temperate environments.

Journal of Coastal Research↗
USGS1978

Recognition of oxidized sulfide minerals as an exploration guide for uranium

The difference in color between tan to red oxidized sandstone and gray reduced sandstone on either side of the reduction-oxidation (redox) interface, which is- the locus of uranium concentration in roll-type deposits, has been noted and used locally as an exploration guide within known uranium districts. Reduced sandstone is characterized in many deposits by the presence of iron sulflde minerals (particularly marcasite and pyrite) that occur as replacements of and overgrowths on iron-titanium oxide minerals and plant debris and as cement of detrital grains. Oxidation of the sulfldes by oxygenated ground water forms yellow to red ferric oxide and ferric hydroxide phases ("limonite") that replace the FeS 2 minerals. Processes other than the oxidation of sulfldes, however, can cause reddening of clastic sediments without the creation of a redox boundary, and so color alone is not a sufficient condition by which to judge the potential for uranium ore in frontier areas. Ferric oxides that form by the oxidation of iron sulflde minerals can be distinguished from other forms of ferric oxide by reflection microscopic examination of polished grain mounts- and polished thin sections'. Diagnostic features of oxidized sulfldes are limonite pseudomorphs of sulfldes and limonite containing internal textures that mimic characteristic textures of previously sulfldized detrital phases. Recognition of oxidized sulfides by reflection microscopy, then, can distinguish oxidized sandstones, which might have a redox boundary downdip and which would therefore be favorable hosts for uranium concentration, from those without such potential.

Journal of Research of the U.S. Geological Survey↗
USGS2023

Time-lapse seafloor surveys reveal how turbidity currents and internal tides in Monterey Canyon interact with the seabed at centimeter-scale

Here we show how ultra-high resolution seabed mapping using new technology can help to understand processes that sculpt submarine canyons. Time-lapse seafloor surveys were conducted in the axis of Monterey Canyon, ∼50 km from the canyon head (∼1,840 m water depth) over an 18-month period. These surveys comprised 5-cm resolution multibeam bathymetry, 1-cm resolution lidar bathymetry, and 2-mm resolution stereophotographic imagery. Bathymetry data reveal centimeter-scale textures that would be undetectable by more traditional survey methods. Upward-looking Acoustic Doppler Current Profilers at the site recorded the flow character of internal tides and the passage of three turbidity currents, while sediment cores collected from the site record flow deposits. Combined with flow and core data, the bathymetry shows how turbidity currents and internal tides modify the seabed. The turbidity currents drape sediment across the site, infilling bedform troughs and smoothing erosional features carved by the internal tides (e.g., rippled scours). Turbidity currents with speeds of 0.9–3.3 m/s failed to cause notable bedform movement, which is surprising given that flows with similar speeds produced rapid bedform migration elsewhere, including the upper Monterey Canyon. The lack of migration may be related to the character of the underlying substrate or indicate that turbidity currents at the site lack dense, near-bed layers. The scale of scours produced by the internal tides (≤0.7 m/s) approaches the scale of features recorded in the ancient rock record. Thus, these results illustrate how the scale gap between seabed mapping technology and the rock record may eventually be bridged.

California↗
USGS2020

Submarine landslide kinematics derived from high-resolution imaging in Port Valdez, Alaska

Submarine landslides caused by strong ground shaking during the M9.2 1964 Great Alaska earthquake generated a tsunami that destroyed much of the old town of Valdez, Alaska, and was responsible for 32 deaths at that location. We explore structural details of the 1964 landslide deposit, as well as landslide deposits from earlier events, in order to characterize kinematics of the landslide process. We present a new high‐resolution seismic reflection data set that images the 1964 landslide deposit and six pre‐1964 deposits with great detail. These deposits are represented by thick packages (~7–23 m) of debris within >500 m of fjord sedimentation above basement. Internal slide structures are associated with distinctive landslide failure mechanisms, including detailed erosional and depositional features and structures resolved within both landslide blocks and distal debris flow layers. Based on comparisons of deposit volume from subbottom structure and differenced bathymetry, we refine prior interpretations of the source of failed material. New data show evidence for basal erosion and reworking of fjord‐floor sedimentation. Additionally, material comprising the 1964 landslide appears to have been translated and deformed by lateral thrusting, rather than having been sourced entirely from upslope evacuation zones. Taking into account these complexities in depositional patterns, we show variations in slide size through Holocene time and relate the history of landslides to the paleoseismic record. Collectively, these new observations demonstrate that Port Valdez has a repeated history of large submarine landslides, which are likely associated with large megathrust earthquakes.

Alaska↗
USGS2011

OSL dating of a Pleistocene maar: Birket Ram, the Golan heights

Direct dating of maars and their phreatomagmatic deposits is difficult due to the dominance of lithic (host rock) fragments and glassy particles of the juvenile magma. In this paper we demonstrate that optically stimulated luminescence (OSL) dating can be successfully used for age determination of phreatomagmatic deposits. We studied the tuff deposit of Birket Ram, a basanitic maar located at the northern edge of the Golan heights on the western Arabian plate. The maar is underlain by a thick section of Pleistocene basalts, and currently hosts a small lake. It is filled by approximately 90m of lacustrine sediments with radiocarbon ages extrapolated to 108ka at the base. OSL was applied to quartz grains extracted from tuffs and paleosols in order to set the time frame of the phreatomagmatism at the site. A maximum age constraint of 179??13ka was determined for a paleosol that underlies the maar ejecta. Quartz grains from two layers in the tuff section yielded a direct age of 129??6ka for the phreatomagmatic eruption. A younger age of 104??7ka, which was determined for a tuff layer underlying a basaltic flow, was attributed to thermal resetting during the lava emplacement. This was confirmed by an 40Ar/39Ar age of 101??3ka determined on the overlying basalt. The internal consistency of the OSL ages and the agreement with the 40Ar/39Ar age determination as well as with previous estimates demonstrates the potential of OSL for maar dating. ?? 2010 Elsevier B.V.

Journal of Volcanology and Geothermal Research↗
USGS2009

The Pliocene Lost River found to west: Detrital zircon evidence of drainage disruption along a subsiding hotspot track

SHRIMP analysis of U/Pb ages of detrital zircons in twelve late Miocene to Pleistocene sand samples from six drill cores on the Snake River Plain (SRP), Idaho, suggests that an ancestral Lost River system was drained westward along the northern side of the SRP. Neoproterozoic (650 to 740??Ma, Cryogenian) detrital zircon grains from the Wildhorse Creek drainage of the Pioneer Mountains core complex, with a source in 695??Ma orthogneiss, and which are characteristic of the Big Lost River system, are found in Pliocene sand from cores drilled in the central SRP (near Wendell) and western SRP (at Mountain Home). In addition to these Neoproterozoic grains, fluvial sands sourced from the northern margin of the SRP contain detrital zircons with the following ages: 42 to 52??Ma from the Challis magmatic belt, 80 to 100??Ma from the Atlanta lobe of the Idaho batholith, and mixed Paleozoic and Proterozoic ages (1400 to 2000??Ma). In contrast, sands in the Mountain Home Air Base well (MHAB) that contain 155-Ma Jurassic detrital grains with a source in northern Nevada are interpreted to represent an integrated Snake River, with provenance on the southern, eastern and northern sides of the SRP. We propose that late Pliocene and early Pleistocene construction of basaltic volcanoes and rhyolitic domes of the Axial Volcanic Zone of the eastern SRP and the northwest-trending Arco Volcanic Rift Zone (including the Craters of the Moon volcanic center), disrupted the paleo-Lost River drainage, confining it to the Big Lost Trough, a volcanically dammed basin of internal drainage on the Idaho National Laboratory (INL). After the Axial Volcanic Zone and Arco Volcanic Rift Zone were constructed to form a volcanic eruptive and intrusive highland to the southwest, sediment from the Big Lost River was trapped in the Big Lost Trough instead of being delivered by surface streams to the western SRP. Today, water from drainages north of the SRP enters the Snake River Plain regional aquifer through sinks in the Big Lost Trough, and the water resurfaces at Thousand Springs, Idaho, about 195??km to the southwest. Holocene to latest Pliocene samples from drill core in the Big Lost Trough reveal interplay between the glacio-fluvial outwash of the voluminous Big Lost River system and the relatively minor Little Lost River system. A mixed provenance signature is recognized in fine-grained sands deposited in a highstand of a Pleistocene pluvial-lake system. ?? 2009 Elsevier B.V.

Journal of Volcanology and Geothermal Research↗
USGS2010

Resilience and vulnerability of permafrost to climate change

The resilience and vulnerability of permafrost to climate change depends on complex interactions among topography, water, soil, vegetation, and snow, which allow permafrost to persist at mean annual air temperatures (MAATs) as high as +2 °C and degrade at MAATs as low as –20 °C. To assess these interactions, we compiled existing data and tested effects of varying conditions on mean annual surface temperatures (MASTs) and 2 m deep temperatures (MADTs) through modeling. Surface water had the largest effect, with water sediment temperatures being ~10 °C above MAAT. A 50% reduction in snow depth reduces MADT by 2 °C. Elevation changes between 200 and 800 m increases MAAT by up to 2.3 °C and snow depths by ~40%. Aspect caused only a ~1 °C difference in MAST. Covarying vegetation structure, organic matter thickness, soil moisture, and snow depth of terrestrial ecosystems, ranging from barren silt to white spruce (Picea glauca (Moench) Voss) forest to tussock shrub, affect MASTs by ~6 °C and MADTs by ~7 °C. Groundwater at 2–7 °C greatly affects lateral and internal permafrost thawing. Analyses show that vegetation succession provides strong negative feedbacks that make permafrost resilient to even large increases in air temperatures. Surface water, which is affected by topography and ground ice, provides even stronger negative feedbacks that make permafrost vulnerable to thawing even under cold temperatures.

Alaska↗
USGS2008

Coarse-clast ridge complexes of the Caribbean: A preliminary basis for distinguishing tsunami and storm-wave origins

Coastal gravel-ridge complexes deposited on islands in the Caribbean Sea are recorders of past extreme-wave events that could be associated with either tsunamis or hurricanes. The ridge complexes of Bonaire, Jamaica, Puerto Rico (Isla de Mona), and Guadeloupe consist of polymodal clasts ranging in size from sand to coarse boulders that are derived from the adjacent coral reefs or subjacent rock platforms. Ridge-complex morphologies and crest elevations are largely controlled by availability of sediments, clast sizes, and heights of wave runup. The ridge complexes are internally organized, display textural sorting and a broad range of ages including historical events. Some display seaward-dipping beds and ridge-and-swale topography, and some terminate in fans or steep avalanche slopes. Together, the morphologic, sedimentologic, lithostratigraphic, and chronostratigraphic evidence indicates that shore-parallet ridge complexes composed of gravel and sand that are tens of meters wide and several meters thick are primarily storm-constructed features that have accumulated for a few centuries or millennia as a result of multiple high-frequency intense-wave events. They are not entirely the result of one or a few tsunamis as recently reported. Tsunami deposition may account for some of the lateral ridge-complex accretion or boulder fields and isolated blocks that are associated with the ridge complexes. Copyright ?? 2008, SEPM (Society for Sedimentary Geology).

Journal of Sedimentary Research↗
USGS2022

Evidence for fluctuating wind in shaping an ancient Martian dune field: The Stimson formation at the Greenheugh pediment, Gale crater

Temporal fluctuations of wind strength and direction can influence aeolian bedform morphology and orientation, which can be encoded into the architecture of aeolian deposits. These strata represent a direct record of atmospheric processes and can be used to understand ancient Martian atmospheric processes as well as those on Earth. The strata can: give insight to ancient atmospheric circulation, how the atmosphere evolved in response to global changes in habitability, and how ancient processes differ from modern processes. The Stimson formation at the Greenheugh pediment (Gale crater) records evidence of fluctuating wind across multiple temporal scales. The strata can be subdivided into three intervals–Gleann Beag, Ladder, and Edinburgh intervals. Internally, the intervals record changes of dune morphology and orientation, correlatable to wind fluctuations at multiple temporal scales. The basal Gleann Beag interval comprises compound cross-strata, deposited by oblique compound dunes. These dunes record a bimodal wind regime, resulting in net sediment transport toward the north. The Ladder interval records a reversal of sediment transport to the south, where straight-crested simple-dunes shaped by a seasonally variable winds formed. Finally, the Edinburgh interval records sediment transport to the west, where a unimodal wind formed sinuous-crested simple dunes. These observations demonstrate active and variable atmospheric circulation in Gale crater during the accumulation of the Stimson dune field, at multiple temporal scales from seasonally driven winds to much longer time-frames, during the Hesperian. These observations can be used to further understand ancient atmospheric conditions and processes, at a high temporal resolution on Mars.

Journal of Geophysical Research - Planets↗
USGS2008

Environmental presence and persistence of pharmaceuticals: An overview

Emerging contaminants (ECs) in the environment – that is, chemicals with domestic, municipal, industrial, or agricultural sources that are not commonly monitored but may have the potential for adverse environmental effects – is a rapidly growing field of research. The use of “emerging” is not intended to infer that the presence of these compounds in the environment is new. These chemicals have been released into the environment as long as they have been in production or, in the case of hormones and other endogenous compounds, since the rise of animal life. What is emerging is the interest by the scientific and lay communities in the presence of these chemicals in the environment, the analytical capabilities required for detection, and the subtle effects that very small concentrations of these chemicals appear to have on aquatic biota. In December 2006, Environmental Science & Technology devoted an entire special issue (volume 40, number 23) to the topic of ECs, illustrating the increased interest in the subject. Within the EGs, one particular class that has seen a substantial increase in research over the past 10 years is pharmaceuticals and personal-care products (PPCPs). This increased research interest can be demonstrated by several means, including requests for proposals from funding agencies, but the clearest indication of a focused effort to understand the introduction, transformation, and potential health and environmental effects of PPCPs and ECs, in general, is the number of published reports. This increase can be shown by examining six environmental journals that regularly publish PPCP-related papers – Chemosphere , Environmental Science & Technology , Environmental Toxicology and Chemistry , Science of the Total Environment , Water Research , and Water Science and Technology . In 1998 there were 22 papers published on pharmaceuticals, antibiotics, or drugs in these 6 journals; by 2006, this number increased sixfold to 132 papers (Figure 1.1). This growth can be attributed to a number of factors. The presence of pharmaceuticals in surface-water samples from Europe and the United States was documented in several sentinel papers. These ground-breaking works encouraged other scientists to examine the rivers, streams, lakes, and reservoirs in their regions for such chemicals. In addition, the intense public attention paid to news reports on the environmental detections of these chemicals and possible effects of aquatic life has made this issue visible to the wastewater-treatment, drinking-water treatment, and regulatory communities. This has driven the funding bodies associated with these communities to fund studies or request proposals that address the presence, fate, and effects of PPCPs in aquatic systems. The release of the first comprehensive reconnaissance of pharmaceuticals and other wastewater contaminants in the United States provides an example of the intense media interest in this topic. Within 6 days on online publication of this study, 72 newspapers across the United States had published articles describing the results, either locally written or based on international media syndicate reports. There also was substantial concurrent coverage by local and national radio and television outlets, including the Cable News Network, ABC World News Tonight , and National Public Radio. A substantial fraction of these news stories may be attributable to press releases and media briefings prior to publication. However, the interest by television and print journalists in reporting the results of a peer-reviewed journal article to the general public was motivated by the recognition that describing the presence of PPCPs in water supplies would be of interest to the public. To better convey the results of the study published by Koplin et al. to the public, a separate general-interest fact sheet was published to summarize the important points of the study. Because PPCPs are commonly and widely used by individuals, there is likely a preexisting, personal identification with these compounds that does not occur for the wide range of other organic and inorganic contaminants whose presence in the environment has previously been described. This greater public “name recognition” makes itself known through the media to the regulatory and technical community and has prompted interest in sponsoring research that defines the composition and concentrations of PPCPs in potential sources and their fate and effects following relase into the environment. Independent of the drivers that potentially fuel the interest in studies of PPCPs, it is clear that PPCP research has grown beyond surface-water studies to examine issues such as: • Presence in other matrices, such as groundwater, landfill leachates, sediments, and biosolids. • Environmental transport and fate in surface water, groundwater, and soils amended with reclaimed water or biosolids. • PPCP source elucidation, such as wastewater treatment plant (WWTP) effluents, confined animal feeding operations (CAFOs), and aquaculture. • Removal during wastewater and drinking-water treatment. • Effects on aquatic ecosystems, terrestrial ecosystems, and human health. The chapters in this book provide an extensive examination of current environmental pharmaceutical research and are divided into three sections: “Occurrence and Analysis of Pharmaceuticals in the Environment,” “Environment Fate and Transformations of Veterinary Pharmaceuticals,” and “treatment of Pharmaceuticals in Drinking Water and Wastewater.” The purpose of this introductory overview chapter is to outline current (2004-2006) knowledge about the presence and concentration of PPCPs as described in the published literature. Previous reviews should be consulted for discussions on pre-2004 publications. Those reviews will provide the reader with a comprehensive introduction to the topic of PPCPs in the environment. This chapter describes the sources of PPCPs and other organic contaminants often associated with human wastewater into the environment, the range of concentrations present in various environmental compartments, and the potential routes of removal/sequestration. An overview of the sources and fate of veterinary pharmaceuticals will be discussed in Chapter 5, “Fate and Transport of Veterinary Medicines in the Soil Environment.”

Book chapter↗
USGS2024

Genetic origins of a resurging lake whitefish, Coregonus clupeaformis, population in the Detroit River, Laurentian Great Lakes

The Detroit River connects Lake Huron and Lake Erie of the Laurentian Great Lakes. The river once supported a substantial lake whitefish ( Coregonus clupeaformis ) fishery until the early 1900s, when habitat loss, pollution, and overfishing contributed to the collapse of the fishery and loss of spawning populations in the river. In the early 1970s, efforts were initiated to improve water and habitat quality, and in December 2005 a spawning male lake whitefish and viable eggs were collected; the first documented evidence of spawning since 1916. Researchers have tracked the spawning magnitude of the lake whitefish population in the Detroit River since 2005 by assessing the number of eggs deposited on egg mats. Genetic analysis of larval fish hatched from eggs collected in the field between 2005 and 2018 was used to determine the relative contributions of Lake Erie and Lake Huron to the resurging population. Over 80% of the hatched larvae had parents originating from Lake Erie in all the years sampled. The estimated number of full-sibling families sampled at Belle Isle was the same in 2010 and 2014 and varied between 2009 and 2016 at Fighting Island. The estimated number of lake whitefish parents at Fighting Island decreased in the most recent collections possibly due to loss of habitat on spawning reefs due to sedimentation. Our results provide additional evidence that restored spawning habitat in the Detroit River is again being used by lake whitefish and continued reproduction at these sites may improve the Great Lakes portfolio of ecological and genetic diversity.

Detroit River↗
USGS2012

Long-term observations of bottom current and bottom sediment movement on the mid-Atlantic continental shelf

Long-term in situ observations made at three locations on the mid-Atlantic continental shelf during 1975–1976 clearly show intermittent movement of bottom sediment caused by currents, waves, and other forcing mechanisms. In winter, storm-associated bottom currents greater than 30 cm s −1 resuspended and transported sediments. Net water particle excursions during storms were about 20–30 km longshelf and 5–10 km cross-shelf. Wave-induced bottom currents also resuspended sediments during periods of low mean flow. Sediment motion was observed in summer, although bottom conditions were generally tranquil. Significant changes in suspended matter concentration were observed that were only partially related to bottom currents. These changes may have been caused by biological activity or advection. Bottom currents on the mid-Atlantic region of the continental shelf were characterized by a coherent, primarily cross-shelf tidal flow of 5–10 cm s −1 and a low-frequency longshelf component of 5–20 cm s −1 . The longshelf current was coherent over length scales of 100 km at tidal frequencies and for motions with periods greater than 50 hours. For these longer periods the longshelf flow was coherent with wind stress, which implies that winds were a major driving force of the longshelf current. The cross-shelf current was not coherent at stations separated by 100 km except at tidal frequencies. Packets of high-frequency internal waves were observed during stratified conditions in summer with bottom currents as large as 20 cm s −1 .

Mid-Atlantic continental shelf↗