Geology topics

P.R. Renne

Publications and source records attributed to P.R. Renne.

6 recordsLinked to original sources

USGS2023

First observation of the ground-state electron-capture of 40K

Potassium-40 is a widespread, naturally occurring isotope whose radioactivity impacts estimated geological ages spanning billions of years, nuclear structure theory, and subatomic rare-event searches—including those for dark matter and neutrinoless double-beta decay. The decays of this long-lived isotope must be precisely known for its use as a geochronometer, and to account for its presence in low-background experiments. There are several known decay modes for potassium-40, but a predicted electron-capture decay directly to the ground state of argon-40 has never been observed. The existence of this decay mode impacts several fields, while theoretical predictions span an order of magnitude. Here we report on the first, successful observation of this rare decay mode, obtained by the KDK (potassium decay) Collaboration using a novel combination of a low-threshold x-ray detector surrounded by a tonne-scale, high-efficiency γ -ray tagger at Oak Ridge National Laboratory. A blinded analysis reveals a distinctly nonzero ratio of intensities of ground-state electron-captures ( I EC 0 ) over excited-state ones ( I EC ∗ ) of I EC 0 / I EC ∗ = 0.0095 stat ± 0.0022 sys ± 0.0010 (68% CL), with the null hypothesis rejected at 4 σ [Stukel et al. , Phys. Rev. Lett. 131 , 052503 (2023) ]. In terms of branching ratio, this unambiguous signal yields I EC 0 = 0.098 % stat ± 0.023 % sys ± 0.010 % , roughly half of the commonly used prediction. This first observation of a third-forbidden unique electron capture improves our understanding of low-energy backgrounds in dark-matter searches and has implications for nuclear-structure calculations. For example, a shell-model based theoretical estimate for the neutrinoless double-beta decay half-life of calcium-48 is increased by a factor of 7 + 3 − 2 . Our nonzero measurement shifts geochronological ages by up to a percent; implications are illustrated for Earth and solar system chronologies.

Physical Review C↗

USGS2023

Rare 40K decay with implications for fundamental physics and geochronology

Potassium-40 is a widespread, naturally occurring isotope whose radioactivity impacts subatomic rare-event searches, nuclear structure theory, and estimated geological ages. A predicted electron-capture decay directly to the ground state of argon-40 has never been observed. The KDK (potassium decay) collaboration reports strong evidence of this rare decay mode. A blinded analysis reveals a nonzero ratio of intensities of ground-state electron-captures ( I EC 0 ) over excited-state ones ( I EC ∗ ) of I EC 0 / I EC ∗ = 0.0095 stat ± 0.0022 sys ± 0.0010 (68% C.L.), with the null hypothesis rejected at 4 σ . In terms of branching ratio, this signal yields I EC 0 = 0.098 % stat ± 0.023 % sys ± 0.010 % , roughly half of the commonly used prediction, with consequences for various fields [L. Hariasz et al. , companion paper, Phys. Rev. C 108 , 014327 (2023) ].

Physical Review Letters↗

USGS2009

Magnetostratigraphic correlations of Permian-Triassic marine-to-terrestrial sections from China

We have studied three Permian–Triassic (PT) localities from China as part of a combined magnetostratigraphic, 40 Ar/ 39 Ar and U–Pb radioisotopic, and biostratigraphic study aimed at resolving the temporal relations between terrestrial and marine records across the Permo-Triassic boundary, as well as the rate of the biotic recovery in the Early Triassic. The studied sections from Shangsi (Sichuan Province), Langdai (Guihzou Province), and the Junggar basin (Xinjiang Province), span marine, paralic, and terrestrial PT environments, respectively. Each of these sections was logged in detail in order to place geochronologic, paleomagnetic, geochemical, conodont and palynologic samples within a common stratigraphic context. Here we present rock-magnetic, paleomagnetic and magnetostratigraphic results from the three localities. At Shangsi, northern Sichuan Province, we sampled three sections spanning Permo-Triassic marine carbonates. Magnetostratigraphic results from the three sections indicate that the composite section contains at least eight polarity chrons and that the PT boundary occurs within a normal polarity chron a short distance above the mass extinction level and a reversed-to-normal (R-N) polarity reversal. Furthermore, the onset of the Illawarra mixed interval lies below the sampled section indicating that the uppermost Permian Changhsingian and at least part of the Wuchiapingian stages postdate the end of the Kiaman Permo-Carboniferous Reversed Superchron. At Langdai, Guizhou Province, we studied magnetostratigraphy of PT paralic mudstone and carbonate sediments in two sections. The composite section spans an R-N polarity sequence. Section-mean directions pass a fold test at the 95% confidence level, and the section-mean poles are close to the mean PT pole for the South China block. Based on biostratigraphic constraints, the R-N transition recorded at Langdai is consistent with that at Shangsi and demonstrates that the PT boundary occurred within a normal polarity chron a short distance above the mass extinction level. In the southern Junggar basin, Xinjiang Province, in northwest China, we determined the magnetostratigraphy of three sections of a terrestrial sequence. Normal and reversed polarity directions are roughly antipodal, and magnetostratigraphies from the three sections are highly consistent. Combined bio- and magneto-stratigraphy used to correlate this sequence to other PT sequences suggests that the previously-proposed biostratigraphic PT boundary in the Junggar sections was most likely misplaced by earlier workers suggesting that further work is necessary to confidently place the PT boundary there.

Journal of Asian Earth Sciences↗

USGS2001

The Permian-Triassic boundary & mass extinction in China

The first appearance of Hindeodus parvus (Kozur & Pjatakova) at the Permian-Triassic (P-T) GSSP level (base of Bed 27c) at Meishan is here confirmed. Hindeodus changxingensis Wang occurs from Beds 26 to 29 at Meishan and appears to be restricted to the narrow boundary interval immediately above the main mass extinction level in Bed 25. It is suggested that this species is therefore a valuable P-T boundary interval index taxon. Our collections from the Shangsi section confirm that the first occurrence of Hindeodus parvus in that section is about 5 in above the highest level from which a typical Permian fauna is recovered. This may suggest that that some section may be missing at Meishan. The age of the currently defined Permian-Triassic Boundary is estimated by our own studies and a reassessment of previous worker's data at c. 253 Ma, slightly older than our IDTIMS 206Pb/238U age of 252.5 ??0.3 Ma for Bed 28, just 8 cm above the GSSP boundary (Mundil et al., 2001). The age of the main mass extinction, at the base of Bed 25 at Meishan, is estimated at slightly older than 254 Ma based on an age of >254 Ma for the Bed 25 ash. Regardless of the absolute age of the boundary, it is evident that the claimed <165,000 y short duration for the negative carbon isotope excursion at the P-T boundary (Bowring et al., 1998) cannot be confirmed. Purportedly extraterrestrial fullerenes at the boundary (Hecker et al., 2001) have equivocal significance due to their chronostratigraphic non-uniqueness and their occurrence in a volcanic ash.

Episodes↗

USGS1996

The 40Ar/39Ar and K/Ar dating of lavas from the Hilo 1-km core hole, Hawaii Scientific Drilling Project

Mauna Kea lava flows cored in the Hilo hole range in age from <200 ka to about 400 ka based on 40 Ar/ 39 Ar incremental heating and K‐Ar analyses of 16 groundmass samples and one coexisting plagioclase. The lavas, all subaerially deposited, include a lower section consisting only of tholeiitic basalts and an upper section of interbedded alkalic, transitional tholeiitic, and tholeiitic basalts. The lower section has yielded predominantly complex, discordant 40 Ar/ 39 Ar age spectra that result from mobility of 40 Ar and perhaps K, the presence of excess 40 Ar, and redistribution of 39 Ar by recoil. Comparison of K‐Ar ages with 40 Ar/ 39 Ar integrated ages indicates that some of these samples have also lost 39 Ar. Nevertheless, two plateau ages of 391 ± 40 and 400 ± 26 ka from deep in the hole, combined with data from the upper section, show that the tholeiitic section accumulated at an average rate of about 7 to 8 m/kyr and has a mean recurrence interval of 0.5 kyr/flow unit. Samples from the upper section yield relatively precise 40 Ar/ 39 Ar plateau and isotope correlation ages of 326 ± 23, 241 ± 5, 232 ± 4, and 199 ± 9 ka for depths of −415.7 m to −299.2 m. Within their uncertainty, these ages define a linear relationship with depth, with an average accumulation rate of 0.9 m/kyr and an average recurrence interval of 4.8 kyr/flow unit. The top of the Mauna Kea sequence at −280 m must be older than the plateau age of 132 ± 32 ka, obtained for the basal Mauna Loa flow in the corehole. The upward decrease in lava accumulation rate is a consequence of the decreasing magma supply available to Mauna Kea as it rode the Pacific plate away from its magma source, the Hawaiian mantle plume. The age‐depth relation in the core hole may be used to test and refine models that relate the growth of Mauna Kea to the thermal and compositional structure of the mantle plume.

Journal of Geophysical Research B: Solid Earth↗

USGS1995

High-3He plume origin and temporal-spatial evolution of the Siberian flood basalts

An olivine nephelinite from the lower part of a thick alkalic ultrabasic and mafic sequence of volcanic rocks of the northeastern part of the Siberian flood basalt province (SFBP) yielded a 40 Ar/ 39 Ar plateau age of 253.3 ± 2.6 million years, distinctly older than the main tholeiitic pulse of the SFBP at 250.0 million years. Olivine phenocrysts of this rock showed 3 He/ 4 He ratios up to 12.7 times the atmospheric ratio; these values suggest a lower mantle plume origin. The neodymium and strontium isotopes, rare earth element concentration patterns, and cerium/lead ratios of the associated rocks were also consistent with their derivation from a near-chondritic, primitive plume. Geochemical data from the 250-million-year-old volcanic rocks higher up in the sequence indicate interaction of this high- 3 He SFBP plume with a suboceanic-type upper mantle beneath Siberia.

Science↗