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Geology topics

Gerard Rocher-Ros

Publications and source records attributed to Gerard Rocher-Ros.

4 recordsLinked to original sources

Global methane budget 2000-2020

Understanding and quantifying the global methane (CH 4 ) budget is important for assessing realistic pathways to mitigate climate change. CH 4 is the second most important human-influenced greenhouse gas in terms of climate forcing after carbon dioxide (CO 2 ), and both emissions and atmospheric concentrations of CH 4 have continued to increase since 2007 after a temporary pause. The relative importance of CH 4 emissions compared to those of CO 2 for temperature change is related to its shorter atmospheric lifetime, stronger radiative effect, and acceleration in atmospheric growth rate over the past decade, the causes of which are still debated. Two major challenges in quantifying the factors responsible for the observed atmospheric growth rate arise from diverse, geographically overlapping CH 4 sources and from the uncertain magnitude and temporal change in the destruction of CH 4 by short-lived and highly variable hydroxyl radicals (OH). To address these challenges, we have established a consortium of multidisciplinary scientists under the umbrella of the Global Carbon Project to improve, synthesise, and update the global CH 4 budget regularly and to stimulate new research on the methane cycle. Following Saunois et al. (2016, 2020), we present here the third version of the living review paper dedicated to the decadal CH 4 budget, integrating results of top-down CH 4 emission estimates (based on in situ and Greenhouse Gases Observing SATellite (GOSAT) atmospheric observations and an ensemble of atmospheric inverse-model results) and bottom-up estimates (based on process-based models for estimating land surface emissions and atmospheric chemistry, inventories of anthropogenic emissions, and data-driven extrapolations). We present a budget for the most recent 2010–2019 calendar decade (the latest period for which full data sets are available), for the previous decade of 2000–2009 and for the year 2020. The revision of the bottom-up budget in this 2025 edition benefits from important progress in estimating inland freshwater emissions, with better counting of emissions from lakes and ponds, reservoirs, and streams and rivers. This budget also reduces double counting across freshwater and wetland emissions and, for the first time, includes an estimate of the potential double counting that may exist (average of 23 Tg CH 4 yr −1 ). Bottom-up approaches show that the combined wetland and inland freshwater emissions average 248 [159–369] Tg CH 4 yr −1 for the 2010–2019 decade. Natural fluxes are perturbed by human activities through climate, eutrophication, and land use. In this budget, we also estimate, for the first time, this anthropogenic component contributing to wetland and inland freshwater emissions. Newly available gridded products also allowed us to derive an almost complete latitudinal and regional budget based on bottom-up approaches. For the 2010–2019 decade, global CH 4 emissions are estimated by atmospheric inversions (top-down) to be 575 Tg CH 4 yr −1 (range 553–586, corresponding to the minimum and maximum estimates of the model ensemble). Of this amount, 369 Tg CH 4 yr −1 or ∼ 65 % is attributed to direct anthropogenic sources in the fossil, agriculture, and waste and anthropogenic biomass burning (range 350–391 Tg CH 4 yr −1 or 63 %–68 %). For the 2000–2009 period, the atmospheric inversions give a slightly lower total emission than for 2010–2019, by 32 Tg CH 4 yr −1 (range 9–40). The 2020 emission rate is the highest of the period and reaches 608 Tg CH 4 yr −1 (range 581–627), which is 12 % higher than the average emissions in the 2000s. Since 2012, global direct anthropogenic CH 4 emission trends have been tracking scenarios that assume no or minimal climate mitigation policies proposed by the Intergovernmental Panel on Climate Change (shared socio-economic pathways SSP5 and SSP3). Bottom-up methods suggest 16 % (94 Tg CH 4 yr −1 ) larger global emissions (669 Tg CH 4 yr −1 , range 512–849) than top-down inversion methods for the 2010–2019 period. The discrepancy between the bottom-up and the top-down budgets has been greatly reduced compared to the previous differences (167 and 156 Tg CH 4 yr −1 in Saunois et al. (2016, 2020) respectively), and for the first time uncertainties in bottom-up and top-down budgets overlap. Although differences have been reduced between inversions and bottom-up, the most important source of uncertainty in the global CH 4 budget is still attributable to natural emissions, especially those from wetlands and inland freshwaters. The tropospheric loss of methane, as the main contributor to methane lifetime, has been estimated at 563 [510–663] Tg CH 4 yr −1 based on chemistry–climate models. These values are slightly larger than for 2000–2009 due to the impact of the rise in atmospheric methane and remaining large uncertainty ( ∼ 25 %). The total sink of CH 4 is estimated at 633 [507–796] Tg CH 4 yr −1 by the bottom-up approaches and at 554 [550–567] Tg CH 4 yr −1 by top-down approaches. However, most of the top-down models use the same OH distribution, which introduces less uncertainty to the global budget than is likely justified. For 2010–2019, agriculture and waste contributed an estimated 228 [213–242] Tg CH 4 yr −1 in the top-down budget and 211 [195–231] Tg CH 4 yr −1 in the bottom-up budget. Fossil fuel emissions contributed 115 [100–124] Tg CH 4 yr −1 in the top-down budget and 120 [117–125] Tg CH 4 yr −1 in the bottom-up budget. Biomass and biofuel burning contributed 27 [26–27] Tg CH 4 yr −1 in the top-down budget and 28 [21–39] Tg CH 4 yr −1 in the bottom-up budget. We identify five major priorities for improving the CH 4 budget: (i) producing a global, high-resolution map of water-saturated soils and inundated areas emitting CH 4 based on a robust classification of different types of emitting ecosystems; (ii) further development of process-based models for inland-water emissions; (iii) intensification of CH 4 observations at local (e.g. FLUXNET-CH 4 measurements, urban-scale monitoring, satellite imagery with pointing capabilities) to regional scales (surface networks and global remote sensing measurements from satellites) to constrain both bottom-up models and atmospheric inversions; (iv) improvements of transport models and the representation of photochemical sinks in top-down inversions; and (v) integration of 3D variational inversion systems using isotopic and/or co-emitted species such as ethane as well as information in the bottom-up inventories on anthropogenic super-emitters detected by remote sensing (mainly oil and gas sector but also coal, agriculture, and landfills) to improve source partitioning.

Earth System Science Data

The North American greenhouse gas budget: Emissions, removals, and integration for CO2, CH4, and N2O (2010–2019): Results From the Second REgional Carbon Cycle Assessment and Processes Study (RECCAP2)

Accurate accounting of greenhouse-gas (GHG) emissions and removals is central to tracking progress toward climate mitigation and for monitoring potential climate-change feedbacks. GHG budgeting and reporting can follow either the Intergovernmental Panel on Climate Change methodologies for National Greenhouse Gas Inventory (NGHGI) reporting or use atmospheric-based “top-down” (TD) inversions or process-based “bottom-up” (BU) approaches. To help understand and reconcile these approaches, the Second REgional Carbon Cycle Assessment and Processes study (RECCAP2) was established to quantify GHG emissions and removals for carbon dioxide (CO 2 ), methane (CH 4 ) and nitrous oxide (N 2 O), for ten-land and five-ocean regions for 2010–2019. Here, we present the results for the North American land region (Canada, the United States, Mexico, Central America and the Caribbean). For 2010–2019, the NGHGI reported total net-GHG emissions of 7,270 TgCO 2 -eq yr −1 compared to TD estimates of 6,132 ± 1,846 TgCO 2 -eq yr −1 and BU estimates of 9,060 ± 898 TgCO 2 -eq yr −1 . Reconciling differences between the NGHGI, TD and BU approaches depended on (a) accounting for lateral fluxes of CO 2 along the land-ocean-aquatic continuum (LOAC) and trade, (b) correcting land-use CO 2 emissions for the loss-of-additional-sink capacity (LASC), (c) avoiding double counting of inland water CH 4 emissions, and (d) adjusting area estimates to match the NGHGI definition of the managed-land proxy. Uncertainties remain from inland-water CO 2 evasion, the conversion of nitrogen fertilizers to N 2 O, and from less-frequent NGHGI reporting from non-Annex-1 countries. The RECCAP2 framework plays a key role in reconciling independent GHG-reporting methodologies to support policy commitments while providing insights into biogeochemical processes and responses to climate change.

Global Biogeochemical Cycles

Global methane emissions from rivers and streams

Methane (CH 4 ) is a potent greenhouse gas and its concentrations have tripled in the atmosphere since the industrial revolution. There is evidence that global warming has increased CH 4 emissions from freshwater ecosystems 1 , 2 , providing positive feedback to the global climate. Yet for rivers and streams, the controls and the magnitude of CH 4 emissions remain highly uncertain 3 , 4 . Here we report a spatially explicit global estimate of CH 4 emissions from running waters, accounting for 27.9 (16.7–39.7) Tg CH 4 per year and roughly equal in magnitude to those of other freshwater systems 5 , 6 . Riverine CH 4 emissions are not strongly temperature dependent, with low average activation energy ( E M = 0.14 eV) compared with that of lakes and wetlands ( E M = 0.96 eV) 1 . By contrast, global patterns of emissions are characterized by large fluxes in high- and low-latitude settings as well as in human-dominated environments. These patterns are explained by edaphic and climate features that are linked to anoxia in and near fluvial habitats, including a high supply of organic matter and water saturation in hydrologically connected soils. Our results highlight the importance of land–water connections in regulating CH 4 supply to running waters, which is vulnerable not only to direct human modifications but also to several climate change responses on land.

Nature

GRiMeDB: The Global River Database Methane Database of concentrations and fluxes

Despite their small spatial extent, fluvial ecosystems play a significant role in processing and transporting carbon in aquatic networks, which results in substantial emission of methane ( CH 4 ) into the atmosphere. For this reason, considerable effort has been put into identifying patterns and drivers of CH 4 concentrations in streams and rivers and estimating fluxes to the atmosphere across broad spatial scales. However, progress toward these ends has been slow because of pronounced spatial and temporal variability of lotic CH 4 concentrations and fluxes and by limited data availability across diverse habitats and physicochemical conditions. To address these challenges, we present a comprehensive database of CH 4 concentrations and fluxes for fluvial ecosystems along with broadly relevant and concurrent physical and chemical data. The Global River Methane Database (GriMeDB; https://doi.org/10.6073/pasta/f48cdb77282598052349e969920356ef , Stanley et al., 2023) includes 24 024 records of CH 4 concentration and 8205 flux measurements from 5029 unique sites derived from publications, reports, data repositories, unpublished data sets, and other outlets that became available between 1973 and 2021. Flux observations are reported as diffusive, ebullitive, and total CH 4 fluxes, and GriMeDB also includes 17 655 and 8409 concurrent measurements of concentrations and 4444 and 1521 fluxes for carbon dioxide ( CO 2 ) and nitrous oxide ( N 2 O ), respectively. Most observations are date-specific (i.e., not site averages), and many are supported by data for 1 or more of 12 physicochemical variables and 6 site variables. Site variables include codes to characterize marginal channel types (e.g., springs, ditches) and/or the presence of human disturbance (e.g., point source inputs, upstream dams). Overall, observations in GRiMeDB encompass the broad range of the climatic, biological, and physical conditions that occur among world river basins, although some geographic gaps remain (arid regions, tropical regions, high-latitude and high-altitude systems). The global median CH 4 concentration (0.20 µmol L −1 ) and diffusive flux (0.44 mmol m -2 d -1 ) in GRiMeDB are lower than estimates from prior site-averaged compilations, although ranges (0 to 456 µmol L −1 and − 136 to 4057 mmol m -2 d -1 ) and standard deviations (10.69 and 86.4) are greater for this larger and more temporally resolved database. Available flux data are dominated by diffusive measurements despite the recognized importance of ebullitive and plant-mediated CH 4 fluxes. Nonetheless, GriMeDB provides a comprehensive and cohesive resource for examining relationships between CH 4 and environmental drivers, estimating the contribution of fluvial ecosystems to CH 4 emissions, and contextualizing site-based investigations.

Earth System Science Data